Villains in Japanese animation with expressive features and symbolism not always found in other forms of animation. Anime characters (either heroes or villains) are depicted with traits more realistic and/or less cartoonish, especially when compared to Western media. This often overlaps with Manga Villains due to manga being adapted into anime and vice versa.
IMPORTANT: Do NOT add Villains from Western animation, as they belong in Cartoon Villains, regardless of whether or not they were anime-inspired or anime-esque, though they might be considered characters from anime imitations (i.e. The Boondocks, Avatar: The Last Airbender, The Legend of Korra, Castlevania, RWBY, Ōban Star-Racers).
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- A (Bungo Stray Dogs)
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- A-Laws
- Aaron (The Aristocrat's Otherworldly Adventure)
- Aaroniero Arruruerie
- Abaddon (Seraph of the End)
- Abdul Hakim
- Abdullah (Kinnikuman)
- Abel (Fairy Tail)
- Abel (Saint Seiya)
- Abel Bluefield
- Aber Rindt
- Abidos the Third
- Abil
- Abirama Redder
- Abo
- Abrego
- Absalom (One Piece)
- Abyss Razor
- Abyss Trinity
- Abyssal Fleet
- Abzu
- Accelerator
- Ace (TwinBee)
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- Ace Killer (Netflix)
- Achilles (Cyborg 009)
- Achilles (Mazinger)
- Acidwire
- Acnologia
- Acqua of the Back
- Acro
- Acrobatic Silky
- Ada
- Adam (Black Cat)
- Adam (Evangelion)
- Adam (NieR:Automata)
- Adam Arclight
- Adam Smasher
- Adam Weishaupt
- Adamas (Record of Ragnarok)
- Adamski
- Adiane the Elegant
- Admiral Haruki Kusakabe
- Admiral Perry
- Admiral Rooster Metal
- Adolf Hitler (Dragon Ball)
- Adolf Hitler (Drifters)
- Adolf Hitler (Fullmetal Alchemist)
- Adon Coborlwitz
- Adonis (The Kingdoms of Ruin)
- ADR-01: Jeri Type
- Aegaeon
- Aegir
- Aeos (Dragon Ball)
- Aerodactyl
- Afro Droid
- Agata
- Agent Eekhout
- Agents of DIO
- Agnese Forces
- Agnese Sanctis
- Agni (Record of Ragnarok)
- Ahbmad Saluja
- Ahide Alobo Agatze
- Ai (Yu-Gi-Oh!)
- Ai Imari
- Ai Magase
- Aichi Sendou
- Aiguille Delaz
- Aikawa
- Ail & An
- Aileen Rao
- Aina Sahalin
- Aine
- Ainz Ooal Gown
- Airborne Unit
- Aircraft Carrier Princess
- Airfield Princess
- Airi Himekawa
- AirMan.EXE
- Airzel
- Aisrehdar
- Aisslinger Wernarr
- Aiwass
- Aizam
- Ajeel Ramal
- Ak-Baba
- Aka (Dragon Ball)
- Akagi (Azur Lane)
- Akaginu
- Akahoshi
- Akai (Yozakura Family)
- Akai and Kanie
- Akainu
- Akakabuto
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- Akamimi
- Akane Hiyama
- Akane Shinjo
- Akasha Shishidou (Corpse Princess)
- Akashic
- Akaspetchi & Pipospetchi
- Akatsuki (Chivalry of a Failed Knight)
- Akatsuki (Naruto)
- Akaza
- Akechi Mitsuhide
- Akemi Hinazuki
- Akemi Miyano
- Akemi Nakajima
- Aki Honda
- Aki Myojin
- Aki Tsukino
- Akihiko Kayaba
- Akihiro Kanou
- Akihiro Kurata
- Akiko Yonehara
- Akio Ohtori
- Akira (Akira)
- Akira Mado
- Akira Otoishi
- Akira Takaoka
- Akito Hyuga
- Akito Sohma (Fruits Basket 2001)
- Akito Sohma (Fruits Basket)
- Akoya Matama
- Akudaikan
- Akuma (Street Fighter)
- Akuma Shogun
- Akura-Ou
- Akācho
- Alala
- Alan Gabriel
- Alan Sylvasta
- Alaskan Base Officer
- Alastor (Viewtiful Joe)
- Alauda Hafez
- Alba
- Albatross Sanctos
- Albedo (Overlord)
- Alberich XIII
- Albert de Blois
- Albert James Moriarty
- Albert Maverick
- Albert Yamada
- Albertine
- Albinass
- Aldegor
- Aldra
- Aldrich (The Seven Deadly Sins)
- Aleister Chamber
- Aleister Crowley (A Certain Magical Index)
- Alejandro Corner
- Alekteus
- Alessi
- Alex & Mueller
- Alex Rosewater
- Alexander Anderson
- Alexandryu
- Alexei Barnes Alderp
- Alexei Dionia
- Alexis Leskinen
- Alexis • Kerib
- Alfred, Duke of Meinz
- Alfried Gallant
- Ali Al-Saachez
- Aliana
- Alicia Lohmeyer
- Alien Adacic
- Alien Head Suckers
- Alien Pedan (Netflix)
- Alien Sheik
- Alien Slave Boss
- Alina Gray (anime)
- Alioth (Devil Survivor 2)
- Alito
- All For One
- All-Devouring Narwhal
- Allen (The White Mage Who was Banished From the Hero's Party is Picked Up by an S-Rank Adventurer: This White Mage is Too Out of the Ordinary!)
- Allium Gyojan
- Allomon
- Alois Trancy
- Alpha Richter
- Alphamon
- Alphard al-Asha
- Altair (Re:Creators)
- Alucard (Hellsing)
- Alucard (Rosario+Vampire)
- Alus
- Aluze
- Alva (Arifureta)
- Alva (Pokémon)
- Am (Star Wars Visions)
- Amachi (Naruto)