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Phenology shifts influence regional climate by altering energy, and water fluxes through biophysical processes. However, a quantitative understanding of the phenological control on vegetation’s biophysical feedbacks to regional climate remains elusive. Using long-term remote sensing observations and Weather Research and Forecasting (WRF) model simulations, we investigated vegetation phenology changes from 2003 to 2020 and quantified their biophysical controls on the regional climate in Northeast China. Our findings elucidated that earlier green-up contributed to a prolonged growing season in forests, while advanced green-up and delayed dormancy extended the growing season in croplands. This prolonged presence and increased maximum green cover intensified climate-vegetation interactions, resulting in more significant surface cooling in croplands compared to forests. Surface cooling from forest phenology changes was prominent during May’s green-up (-0.53 ± 0.07 °C), while crop phenology changes induced cooling throughout the growing season, particularly in June (-0.47 ± 0.15 °C), July (-0.48 ± 0.11 °C), and September (-0.28 ± 0.09 °C). Furthermore, we unraveled the contributions of different biophysical pathways to temperature feedback using a two-resistance attribution model, with aerodynamic resistance emerging as the dominant factor. Crucially, our findings underscored that the land surface temperature (LST) sensitivity, exhibited substantially higher values in croplands rather than temperate forests. These strong sensitivities, coupled with the projected continuation of phenology shifts, portend further growing season cooling in croplands. These findings contribute to a more comprehensive understanding of the intricate feedback mechanisms between vegetation phenology and surface temperature, emphasizing the significance of vegetation phenology dynamics in shaping regional climate pattern and seasonality.

A new frequency-stepped Doppler backscattering (DBS) system has been integrated into a real-time steerable electron cyclotron heating launcher system to simultaneously probe local background turbulence (f < 10 MHz) and high-frequency (20–550 MHz) density fluctuations in the DIII-D tokamak. The launcher allows for 2D steering (horizontally and vertically) over wide angular ranges to optimize probe location and wavenumber response. The vertical steering can be optimized during a discharge in real time. The new DBS system employs a programmable frequency synthesizer with adjustable dwell time as a source to launch either O or X-mode polarized millimeter waves. This system can step in real-time over the entire E-band frequency range (60–90 GHz). This combination of capabilities allows for the diagnosis of the complex internal spatial structure of high power (>200 kW) helicon waves (476 MHz) injected from an external antenna during helicon current drive experiments in DIII-D. Broadband density fluctuations around the helicon frequency are observed during real-time scans of measurement location and wavenumber during these experiments. Analysis indicates that these broadband high-frequency fluctuations are a result of backscattering of the DBS millimeter-wave probe beam from plasma turbulence modulated by the helicon wave. It is observed that background turbulence is effectively locally “tagged” with the helicon wave electric field, forming images of the turbulent spectrum in the overall density fluctuation spectrum that appear as high-frequency sidebands of the turbulence. These observations of background turbulence and high-frequency fluctuations open up the possibility of monitoring local helicon wave amplitude by comparing the high-frequency signal amplitude to the simultaneously measured background turbulence. In combination with the real-time measurement location and wavenumber scanning capabilities (offered by real-time frequency-stepping and steering), this allows rapid determination of the spatial distribution of the helicon wave power during steady-state plasma operation.

We report an exploratory study of the structure-dependent electromagnetic radiative corrections to unique first-forbidden nuclear beta decays. We show that the insertion of angular momentum into the nuclear matrix element by the virtual or real photon exchange opens up the decay at vanishing nuclear recoil momentum which was forbidden at tree level, leading to a dramatic change in the decay spectrum not anticipated in existing studies. We discuss its implications for precision tests on the standard model and searches for new physics.

The high pressure behavior of hydrazine, N₂H₄, has been investigated to 50 GPa at room temperature using infrared and Raman spectroscopy to explore pressure induced phase transitions and changes in hydrogen bonding. Three solid–solid phase transitions were detected at 11, 21, and 32 GPa on room temperature compression through dramatic changes in the lattice vibration and N–H stretching regions with increasing pressure in both measurement techniques. The transition to phase IV, which appears at 32 GPa, exhibits increased hydrogen bonding with significant hysteresis, persisting to 9 GPa on decompression. This work presents a detailed analysis of the pressure dependence of mode shifts and calculations of mode Grüneisen parameters as well as a determination of an approximate thermodynamic Grüneisen parameter. We compare these results to the behavior of other small molecular materials such as ammonia and water and explore the evolution of hydrogen bonding in hydrazine toward the symmetrically hydrogen bonded state, which has previously been suggested by theoretical computations.

The evolution of molecular dynamics (MD) simulations has been intimately linked to that of computing hardware. For decades following the creation of MD, simulations have improved with computing power along the three principal dimensions of accuracy, atom count (spatial scale), and duration (temporal scale). Since the mid-2000s, computer platforms have, however, failed to provide strong scaling for MD, as scale-out central processing unit (CPU) and graphics processing unit (GPU) platforms that provide substantial increases to spatial scale do not lead to proportional increases in temporal scale. Important scientific problems therefore remained inaccessible to direct simulation, prompting the development of increasingly sophisticated algorithms that present significant complexity, accuracy, and efficiency challenges. While bespoke MD-only hardware solutions have provided a path to longer timescales for specific physical systems, their impact on the broader community has been mitigated by their limited adaptability to new methods and potentials. In this work, we show that a novel computing architecture, the Cerebras wafer scale engine, completely alters the scaling path by delivering unprecedentedly high simulation rates up to 1.144 M steps/s for 200 000 atoms whose interactions are described by an embedded atom method potential. This enables direct simulations of the evolution of materials using general-purpose programmable hardware over millisecond timescales, dramatically increasing the space of direct MD simulations that can be carried out. In this paper, we provide an overview of advances in MD over the last 60 years and present our recent result in the context of historical MD performance trends.

Biomolecular interactions are essential in many biological processes, including complex formation and phase separation processes. Coarse-grained computational models are especially valuable for studying such processes via simulation. Here, we present COCOMO2, an updated residue-based coarse-grained model that extends its applicability from intrinsically disordered peptides to folded proteins. This is accomplished with the introduction of a surface exposure scaling factor, which adjusts interaction strengths based on solvent accessibility, to enable the more realistic modeling of interactions involving folded domains without additional computational costs. COCOMO2 was parametrized directly with solubility and phase separation data to improve its performance on predicting concentration-dependent phase separation for a broader range of biomolecular systems compared to the original version. COCOMO2 enables new applications including the study of condensates that involve IDPs together with folded domains and the study of complex assembly processes. COCOMO2 also provides an expanded foundation for the development of multiscale approaches for modeling biomolecular interactions that span from residue-level to atomistic resolution.

Cloud responses to surface-based sources of aerosol perturbation partially depend on how turbulent transport of the aerosol to cloud base affects the spatial and temporal distribution of aerosol. Here, scenarios of plume injection below a marine stratocumulus cloud are modeled using large eddy simulations coupled to a prognostic bulk aerosol and cloud microphysics scheme. Both passive plumes, consisting of an inert tracer, and active plumes are investigated, where the latter are representative of saltwater droplet plumes such as have been proposed for marine cloud brightening. Passive plume scenarios show higher in-plume cloud brightness (relative to out-of-plume) due to the predominant transport of the passive plume tracer from the near-surface to the cloud layer within updrafts. These updrafts rise into brighter areas within the cloud deck, even in the absence of an aerosol perturbation associated with an active plume. Comparing albedo at in-plume to out-of-plume locations associates the inert plume with the brightest cloud locations, without any causal effect of the plume on the cloud. Numerical sensitivities are first assessed to establish a suitable model configuration. Then sensitivity to particle injection rate is investigated. Trade-offs are identified between the number of injected particles and the suppressive effect of droplet evaporation on plume loft and spread. Furthermore, as the near-field in-plume brightening effect does not depend significantly on injection rate given a suitable definition of perturbed versus unperturbed regions of the flow, plume area is a key controlling factor on the overall cloud brightening effect of an aerosol perturbation.

We present a technique to assess the spatial aberration content of a focused multi-terawatt laser when fired at full power. This method leverages the direct detection of electrons ponderomotively accelerated from the focal volume formed in a low-pressure gaseous back-fill. Furthermore, our results show that the spatial distribution of emitted electrons exhibits distinct features correlated to the laser aberration type and magnitude. This work represents progress toward the complete and accurate in-situ spatiotemporal characterization of focused high-intensity lasers.

The interference between the atmospheric and solar neutrino oscillation subamplitudes is said to be responsible for CP violation (CPV) in neutrino appearance channels. More precisely, CPV is generated by the interference between the parts of the neutrino oscillation amplitude that are CP even and CP odd: even or odd when the neutrino mixing matrix is replaced with its complex conjugate. This is the CPV interference term, as it gives a contribution to the oscillation probability, the square of the amplitude, which is opposite in sign for neutrinos and antineutrinos and is unique. For this interference to be nonzero, at least two subamplitudes are required. There are, however, other interference terms, which are even under the above exchange, and these are the CP conserving (CPC) interference terms. In this paper, we explore in detail these CPC interference terms and show that they cannot be uniquely defined, as one can move pieces of the amplitude from the atmospheric subamplitude to the solar subamplitude and vice versa. This freedom allows one to move the CPC interference terms around, but does not let you eliminate them completely. We also show that there is a reasonable definition of the atmospheric and solar subamplitudes for the appearance channels such that in neutrino disappearance probability there is no atmospheric-solar CPC interference term. However, with this choice, there is a CPC interference term within the atmospheric sector.

A series of L-mode plasma discharges was performed in the DIII-D tokamak to assess the impact of outer strike point (OSP) position and toroidal magnetic field direction on erosion and core contamination potential of the recently-installed, tungsten-coated Small Angle Slot (SAS-VW) divertor. In one discharge, in-slot emission spectroscopy measured an<48 % increase in the W gross erosion rate when the OSP was moved 3 cm outwards, away from the V-shaped vertex of the slot divertor. However, the effective W yield (erosion rate divided by the incident D flux) was, overall, insensitive to changes in OSP location. Consistently low estimates of the effective W yield based on measurements taken a few cm outwards from the vertex suggest potentially significant C surface contamination. No W emission signal was detected when orienting the toroidal magnetic field such that the ion B×∇B drift direction is pointed away from the X-point. However, measurements of W content in the plasma core for both toroidal magnetic field directions suggest the presence of additional, unmeasured sources of erosion. The difference in the measured core W density with OSP position is much greater than the difference in the measured erosion rates, which may suggest that the leakage of eroded impurities out of the divertor is governed primarily through the parallel ion temperature gradient and friction forces.